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负载型金属催化剂合成表征及催化制备γ-戊内脂的研究

摘要第4-5页
ABSTRACT第5-6页
List of abbreviations第12-13页
CHAPTER 1 INTRODUCTION第13-16页
    1.1 Motivation and Objectives第13-15页
    1.2. Organization of thesis第15-16页
CHAPTER 2 LITERATURE OVERVIEW第16-40页
    2.1 Fuel generation and chemicals production derived from biomass第16-25页
        2.1.1 Definition and composition of biomass第16-21页
        2.1.2 Conversion strategies for lignocellulose to fuels and chemicals第21-25页
            2.1.2.1 Properties of levulinic acid第23-24页
            2.1.2.2 Preparation of levulinic acid from Lignocellulosic biomass第24-25页
    2.2 Potential applications of levulinic acid and its derivatives第25-30页
        2.2.1 Conversion of levulinic acid to valuable compounds第25-27页
        2.2.2 Levulinic acid conversion to γ-Valerolactone第27-30页
            2.2.2.1 Importance and properties of γ-Valerolactone第27-29页
            2.2.2.2 Hydrogenation of Levulinic acid to gamma valerolactone第29-30页
    2.3 Effective H/C ratio and its importance for feedstock and biofuels第30-32页
    2.4 Catalyst Preparation Methods第32-34页
    2.5 Reported Literature of LA hydrogenation to GVL第34-40页
CHAPTER 3 EXPERIMENTAL SECTION第40-52页
    3.1 Materials第40页
    3.2 Pretreatment of Activated carbon and preparation of catalysts第40-42页
        3.2.1 Pre-treatment of Activated carbon supporting materials第40页
        3.2.2 Preparation of non noble metal (Cu, Ni, Mo, Co, W) based catalysts第40-42页
    3.3 Characterization of non noble metal catalysts第42-47页
        3.3.1 Determination of surface area by BET method第42-44页
        3.3.2 Powder X-ray diffraction analysis (XRD)第44-45页
        3.3.3 Transmission Electron Microscopy (TEM)第45-47页
    3.4 Catalytic experiments: Levulinic Acid (LA) Hydrogenation第47-51页
        3.4.1 Catalytic reaction procedure第47-48页
        3.4.2 Products analysis第48-51页
            3.4.2.1 Gas chromatography (GC)第48-50页
            3.4.2.2 Gas chromatograph –Mass Spectrometry (GC-MS)第50-51页
    3.5 Stability test of the metal based catalysts第51-52页
CHAPTER 4 RESULTS AND DISCUSSION第52-71页
    4.1 Catalyst Synthesis and Characterization第52-64页
    4.2 Catalytic activity and Stability of catalysts第64-71页
CHAPTER 5 CONCLUSIONS AND OUTLOOK第71-74页
REFERENCES第74-85页
论文发表及参加科研情况说明第85-86页
ACKNOWLEDGEMENTS第86-88页

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