| Abstract | 第5-10页 |
| 摘要 | 第11-17页 |
| Chapter 1.Introduction | 第17-25页 |
| 1.1 Background and significance | 第17-21页 |
| 1.2 Objectives of the study | 第21页 |
| 1.3 Contents of the study | 第21-22页 |
| 1.4 The organization of this thesis | 第22-23页 |
| 1.5 The innovation of this thesis | 第23-25页 |
| Chapter 2.Literature review | 第25-53页 |
| 2.1 Introduction to antibiotic Sorption studies | 第25-39页 |
| 2.2 Experimental studies for antibiotic adsorption mechanisms | 第39-43页 |
| 2.3 Theoretical calculation of antibiotic and solid particle interaction mechanisms | 第43-47页 |
| 2.4 Adsorption mechanisms of OFL and NOR on solid particles | 第47-51页 |
| 2.5 Key questions to be discussed in this study | 第51-53页 |
| Chapter 3.Adsorption of ofloxacin and norfloxacin on carbon nanotubes:hydrophobicity- and structure-controlled process | 第53-74页 |
| 3.1 Introduction | 第53页 |
| 3.2 Materials and methods | 第53-60页 |
| 3.2.1 Materials | 第53-55页 |
| 3.2.2 Batch adsorption experiments | 第55-56页 |
| 3.2.3 Measurement of solubilities and Kows of OFL and NOR | 第56-57页 |
| 3.2.4 FTIR characterization of OFL or NOR adsorbed adsorbents | 第57-58页 |
| 3.2.5 Detection of OFL and NOR | 第58页 |
| 3.2.6 Data analysis | 第58-60页 |
| 3.3 Results and discussion | 第60-73页 |
| 3.3.1 Stability of OFL and NOR at different concentration | 第60页 |
| 3.3.2 Fitting of sorption isotherms | 第60-65页 |
| 3.3.3 Adsorption as affected by adsorbent surface area and CNT diameters | 第65-67页 |
| 3.3.4 Adsorption as affected by functional groups | 第67-68页 |
| 3.3.5 Different adsorption characteristics between OFL and NOR | 第68-71页 |
| 3.3.6 FTIR spectra of adsorbents before and afer adsorption | 第71-73页 |
| 3.4 Conclusions | 第73-74页 |
| Chapter 4.Adsorption of of loxacin and norfloxacin on carbon nanotubes:pH effect | 第74-88页 |
| 4.1 Introduction | 第74页 |
| 4.2 Materials and methods | 第74-77页 |
| 4.2.1 Materials | 第74-75页 |
| 4.2.2 Batch adsorption experiments | 第75-76页 |
| 4.2.3 Measurement of OFL and NOR solubilities | 第76-77页 |
| 4.2.4 Data analysis | 第77页 |
| 4.3 Results and discussion | 第77-87页 |
| 4.3.1 OFL and NOR solub-lities as affected by pH | 第77-81页 |
| 4.3.2 OFL and NOR adsorption on carbon nanotubes at different pHs | 第81-87页 |
| 4.4 Conclusions | 第87-88页 |
| Chapter 5.Adsorption pf of loxacin and norfloxacin on carbon nanotubes:solubilityand water-methanol cosolvent effects | 第88-114页 |
| 5.1 Introduction | 第88-89页 |
| 5.2 Materials and methods | 第89-94页 |
| 5.2.1 Materials | 第89-91页 |
| 5.2.2 Batch adsorption experiments | 第91-92页 |
| 5.2.3 Measurement of OFL and NOR solubilities | 第92页 |
| 5.2.4 Data analysis | 第92-93页 |
| 5.2.5 DFT computation method | 第93-94页 |
| 5.3 Results and discussion | 第94-111页 |
| 5.3.1 OFL and NOR solubilities as affected by methanol volume fraction | 第94-98页 |
| 5.3.2 OFL and NOR adsorption on carbon nanotubes from water/methanol mixed solvent | 第98-103页 |
| 5.3.3 Strength of hydrogen bond of OFL/NOR and solvent at possible sites | 第103-110页 |
| 5.3.4 Interaction energy of hydration systems | 第110-111页 |
| 5.4 Conclusions | 第111-114页 |
| Chapter 6.Conclusions and prospectives | 第114-117页 |
| 6.1 Conclusions | 第114-115页 |
| 6.2 Perspectives | 第115-117页 |
| Acknowledgements | 第117-119页 |
| Reference | 第119-133页 |
| Appendix 1 List of symbols and abbreviations | 第133-135页 |
| Appendix 2 List of publications and prizes | 第135-136页 |
