| 摘要 | 第3-5页 |
| Abstract | 第5-6页 |
| Chapter 1 Introduction | 第11-26页 |
| 1.1 Background | 第11-13页 |
| 1.2 Fine and coarse particles: general overview | 第13-14页 |
| 1.3 Chemical composition of PM_(2.5) and PM_(10) | 第14-17页 |
| 1.4 Source apportionment with receptor models | 第17-22页 |
| 1.4.1 Modeling with positive matrix factorization | 第19-20页 |
| 1.4.2 Modeling with UNMIX | 第20-21页 |
| 1.4.3 Modeling with principal component analysis | 第21-22页 |
| 1.5 Estimation of infiltration of outdoor particles into indoors | 第22页 |
| 1.6 Estimation of enrichment factors | 第22-23页 |
| 1.7 Potential health effects of exposure to PM_(2.5) and PM_(10) | 第23页 |
| 1.8 Problem statement and scope of study | 第23-24页 |
| 1.8.1 Problem statement | 第23-24页 |
| 1.8.2 study objectives | 第24页 |
| 1.9 Source and main contents | 第24-26页 |
| 1.9.1 Source | 第24-25页 |
| 1.9.2 Main contents | 第25-26页 |
| Chapter 2 Materials and methods | 第26-37页 |
| 2.1 Study area | 第26页 |
| 2.2 Sampling strategy | 第26-27页 |
| 2.3 Chemical analysis | 第27-29页 |
| 2.4 Quality control/quality assurance | 第29-30页 |
| 2.5 Modeling of emission sources | 第30-32页 |
| 2.5.1 Source apportionment with PMF model | 第30-31页 |
| 2.5.2 Modeling with UNMIX | 第31-32页 |
| 2.6 Statistical analysis | 第32-37页 |
| 2.6.1 Estimation of enrichment factors | 第32页 |
| 2.6.2 Non-metric Multi-Dimensional scaling | 第32-33页 |
| 2.6.3 Partial least square (PLS) regression | 第33-34页 |
| 2.6.4 Calculation of PAHs infiltration into indoors | 第34页 |
| 2.6.5 Estimation of cancer risk of PAHs exposure | 第34-37页 |
| Chapter 3 Characteristics and source apportionment of PM_(10) and PM_(2.5) in ambientenvironment | 第37-65页 |
| 3.1 Mass concentrations of PM_(10) and PM_(2.5) in ambient environment | 第37-40页 |
| 3.2 Analysis on chemical composition of PM_(10) and PM_(2.5) | 第40-42页 |
| 3.3 Annual variations of PM_(10) and PM_(2.5) attributed to weather conditions | 第42-46页 |
| 3.4 Seasonal variations of PM_(10) and PM_(2.5) due to meteorological parameters | 第46-48页 |
| 3.5 Intercorrelations among the different species based on Pearson’s correlations | 第48-51页 |
| 3.6 Investigation of distribution patterns of PM_(2.5) and PM_(10) using Linear discriminantanalysis | 第51-54页 |
| 3.7 Source apportionment with PMF and UNMIX | 第54-63页 |
| 3.8 Summary | 第63页 |
| 3.9 本章小结 | 第63-65页 |
| Chapter 4 Findings of inorganic contents of indoor and outdoor PM_(2.5) | 第65-78页 |
| 4.1 Estimation of indoor/outdoor relations of PM_(2.5) and its contents | 第65-68页 |
| 4.2 Evaluation of infiltration and similarity between indoor and outdoor PM_(2.5) usingNMDS | 第68-70页 |
| 4.3 Confirmatory analysis and source apportionment with Partial Least Squareregression | 第70-74页 |
| 4.4 Estimating impact of anthropogenic vs. natural sources | 第74-76页 |
| 4.5 Summary | 第76-77页 |
| 4.6 本章小结 | 第77-78页 |
| Chapter 5 Investigation on polycyclic aromatic hydrocarbons bound to PM_(2.5) inindoor and outdoor air | 第78-108页 |
| 5.1 Total mass levels of PAHs | 第78-81页 |
| 5.2 Concentrations of individual PAH compounds | 第81-85页 |
| 5.3 Estimation of outdoor originated PAHs | 第85-87页 |
| 5.4 Investigating distribution patterns with Linear discriminant analysis | 第87-90页 |
| 5.5 Association between PAHs, meteorological parameters and carbonaceous species | 第90-93页 |
| 5.6 Implications for cancer risk | 第93-100页 |
| 5.6.1 Relative Potency Factor Approach | 第93-96页 |
| 5.6.2 Surrogate marker approach | 第96-100页 |
| 5.7 Source apportionment and estimation of diagnostic isomeric ratios | 第100-106页 |
| 5.8 Summary | 第106-107页 |
| 5.9 本章小结 | 第107-108页 |
| 结论 | 第108-110页 |
| Conclusion | 第110-112页 |
| References | 第112-149页 |
| Papers published in the period of Ph.D. education | 第149-151页 |
| Acknowledgement | 第151-152页 |
| Resume | 第152页 |
