| 摘要 | 第4-7页 |
| ABSTRACT | 第7-10页 |
| Chapter 1: Introduction | 第19-25页 |
| 1.1 Micro Channel Reactors | 第20-22页 |
| 1.1.1 Advantages of Microreactor | 第22页 |
| 1.2 Computational Fluid Dynamics (CFD) | 第22-23页 |
| 1.3 Purpose of research | 第23-25页 |
| Chapter 2: Literature review | 第25-45页 |
| 2.1 Process Intensification-A Brief Overview | 第25-29页 |
| 2.2 Microreactors | 第29-41页 |
| 2.2.1 Description of Microreactors | 第30-34页 |
| 2.2.2 Physical Principles for Chemical Processing in microreactors | 第34-37页 |
| 2.2.3 Micro impinging stream reactor | 第37-40页 |
| 2.2.4 Applications of microreactors in chemical industry | 第40-41页 |
| 2.3 An Introduction of CFD and Ansys Fluent | 第41-45页 |
| 2.3.1 CFD simulation | 第42-44页 |
| 2.3.2 Applications of CFD in engineering | 第44-45页 |
| Chapter 3: Experimental setup and Numerical models | 第45-61页 |
| 3.1 Experimental Apparatus | 第45-47页 |
| 3.2 Materials | 第47页 |
| 3.3 Experimental characterization | 第47-54页 |
| 3.3.1 Competing Chemical Reactions | 第48-49页 |
| 3.3.2 Villermaux-Dushman reaction | 第49-50页 |
| 3.3.3 Reaction Kinetics | 第50-52页 |
| 3.3.4 Segregation Index | 第52-53页 |
| 3.3.5 Principle of Iodine Concentration Measurement | 第53-54页 |
| 3.4 Numerical Modeling in Ansys Fluent | 第54-61页 |
| 3.4.1 Assumptions for the model | 第54页 |
| 3.4.2 Momentum model to study fluid flow patterns | 第54-56页 |
| 3.4.3 Mass transfer modeling | 第56页 |
| 3.4.4 Laminar finite-rate model | 第56-58页 |
| 3.4.5 Eulerian model | 第58-61页 |
| Chapter 4: Flow Patterns and Micromixing: One channel | 第61-79页 |
| 4.1 Multiphase Flow Patterns | 第61-67页 |
| 4.1.1 Intensification zone (Turbulence Contours) | 第61-63页 |
| 4.1.2 Velocity contours of aqueous streams | 第63-64页 |
| 4.1.3 Velocity vectors of aqueous streams | 第64-65页 |
| 4.1.4 Phase contours of aqueous streams | 第65-67页 |
| 4.2 Investigation of Micromixing | 第67-71页 |
| 4.2.1 Micromixing: Xs vs Re | 第67-69页 |
| 4.2.2 Micromixing: Re vs [H_3BO_3] | 第69-70页 |
| 4.2.3 Micromixing: [H~+]=0.04 mol/L, [H~+]=0.05 mol/L and [H~+]=0.06mol/L | 第70-71页 |
| 4.3 Multiphase Flow Patterns: R=2 | 第71-75页 |
| 4.3.1 Intensification zone (Turbulence Contours) | 第71-72页 |
| 4.3.2 Velocity contours of aqueous streams | 第72-73页 |
| 4.3.3 Velocity vectors of aqueous streams | 第73-74页 |
| 4.3.4 Phase contours of aqueous streams | 第74-75页 |
| 4.4 Investigation of Micromixing: R=2 | 第75-77页 |
| 4.4.1 Micromixing: Xs vs Re | 第75-77页 |
| 4.5 Summary | 第77-79页 |
| Chapter 5: Flow Patterns and Micromixing: Two channels | 第79-91页 |
| 5.1 Multiphase Flow Patterns | 第79-86页 |
| 5.1.1 Intensification zone (Turbulence Contours) | 第79-81页 |
| 5.1.2 Velocity contours of aqueous streams | 第81-83页 |
| 5.1.3 Velocity vectors of aqueous streams | 第83-85页 |
| 5.1.4 Phase contours of aqueous streams | 第85-86页 |
| 5.2 Investigation of Micromixing: Xs vs Re | 第86-89页 |
| 5.3 Summary | 第89-91页 |
| Chapter 6: Flow Patterns and Micromixing: Four channels | 第91-99页 |
| 6.1 Multiphase Flow Patterns | 第91-94页 |
| 6.1.1 Intensification zone (Turbulence Contours) | 第91-92页 |
| 6.1.2 Velocity contours of aqueous streams | 第92-93页 |
| 6.1.3 Phase contours of aqueous streams | 第93-94页 |
| 6.2 Investigation of Micromixing: Xs vs Re | 第94-96页 |
| 6.3 Micromixing comparison between One, Two and Four channels | 第96-97页 |
| 6.4 Summary | 第97-99页 |
| Chapter 7: Conclusions | 第99-101页 |
| References | 第101-109页 |
| Acknowledgement | 第109-111页 |
| Publications | 第111-113页 |
| Introduction of Author and Supervisor | 第113-115页 |
| 附件 | 第115-117页 |
